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Hitoshi Mukai | |
Senior Researcher | |
Global Warming Mechanism Research Team | |
Global Environment Division | |
National Institute for Environmental Studies, Ministry of Environment | |
Onogawa 16-2, Tsukuba, Ibaraki, 305-0053, Japan | |
Tel: +81-298-50-2536 Fax: +81-298-50-2569 | |
E-mail: lnmukaih@nies.go.jp |
46,618,000 Yen
(FY 2000; 15,963,000 Yen)
Estimation of carbon dioxide budget in the atmosphere is important issue to asses the future increase of CO2. Growth rate of carbon dioxide was known to change every year. Such a variation may to be related to CO2 budget in nature. In this study, we focused on isotope ratio of carbon dioxide and oxygen concentration change associated with the CO2 growth. These two parameters can give us useful information on the CO2 budget in the atmosphere. To observe these parameters, bottle sampling of background air over the Pacific was carried out with two ships-of-opportunity and by using two monitoring stations (Hateruma Island and Cape Ochi-ishi). Carbon isotope ratio (1995-2000) showed latitudinal gradient and clear seasonal variation with a long-term change. Isotopic budget calculation showed that the CO2 source flux from land biosphere increased in 1998 with a small increase of CO2 sink flux by the ocean, followed by changing to ocean as a source in late 1998. Then land biosphere changed to sink in 1999. Gradually ocean became sink again in 2000.
The 3-year record (Ju1.1997-Jun.2000) and 2-year record (Dec.1998-Nov.2000) of the O2/N2 ratios clearly showed seasonal variations, which inversely co-vary with variations in the CO2 mixing ratio. The changing rates of CO2 mixing ratio and O2/N2 ratio at Hateruma were 2.1±0.1 ppm/yr and -3.7±0.5 ppm/yr, respectively. Assuming that the CO2 production rate by fossil fuel consumption during the same period is 6.6 GtC/yr, these observed CO2 and O2/N2 trends correspond to the land biotic and oceanic uptakes of 1.5±1.0 GtC/yr and 0.9±1.1 GtC/yr, respectively.
Carbon dioxide, Carbon isotope ratio, Oxygen concentration, Pacific ocean, bottle sampling, Hateruma